The matching of the properties of carbon and BN based nanostructures has been carried out. It was studied a strong frequency shifts and changes of the intensities vibrational hands of BN dendritic nanostructures. It was demonstrated the simultaneous manifestation vibrations of nanotubes and diamond-like c-BN. The giant vibrational nonlinearity of BN nanostructures provides an effective nonlinear interaction of vibrational modes with the generation of high-frequency excitations. This fact finds its proof in observation of the glow in the bands of overtones and summary tones.
